Identification

Title

Observations of ice nuclei and heterogeneous freezing in a Western Pacific extratropical storm

Abstract

In situ airborne sampling of refractory black carbon (rBC) particles and Ice Nuclei (IN) was conducted in and near an extratropical cyclonic storm in the western Pacific Ocean during the Pacific Dust Experiment, PACDEX, in the spring of 2007. Airmass origins were from Eastern Asia. Clouds associated primarily with the warm sector of the storm were sampled at various locations and altitudes. Cloud hydrometeors were evaporated by a counterflow virtual impactor (CVI) and the residuals were sampled by a single particle soot photometer (SP2) instrument, a continuous flow diffusion chamber ice nucleus detector (CFDC) and collected for electron microscope analysis. In clouds containing large ice particles, multiple residual particles were observed downstream of the CVI for each ice particle sampled on average. The fraction of rBC compared to total particles in the residual particles increased with decreasing condensed water content, while the fraction of IN compared to total particles did not, suggesting that the scavenging process for rBC is different than for IN. In the warm sector storm midlevels at temperatures where heterogeneous freezing is expected to be significant (here -24 to -29 °C), IN concentrations from ice particle residuals generally agreed with simultaneous measurements of total ice concentrations or were higher in regions where aggregates of crystals were found, suggesting heterogeneous freezing as the dominant ice formation process in the mid levels of these warm sector clouds. Lower in the storm, at warmer temperatures, ice concentrations were affected by aggregation and were somewhat less than measured IN concentrations at colder temperatures. The results are consistent with ice particles forming at storm mid-levels by heterogeneous freezing on IN, followed by aggregation and sedimentation to lower altitudes. Compositional analysis of the aerosol and back trajectories of the air in the warm sector suggested a possible biomass burning source for much of the aerosol. Comparison of the particles from the CFDC with the other aerosol in the residuals of ice particles suggested that the largest portion of IN had similar inferred origins (from biomass burning with minor amounts of rBC) as the other aerosol, but contained slightly elevated amounts of calcium and less influence from sea salt.

Resource type

document

Resource locator

Unique resource identifier

code

http://n2t.net/ark:/85065/d7xp767p

codeSpace

Dataset language

eng

Spatial reference system

code identifying the spatial reference system

Classification of spatial data and services

Topic category

geoscientificInformation

Keywords

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keyword value

Text

originating controlled vocabulary

title

Resource Type

reference date

date type

publication

effective date

2016-01-01T00:00:00Z

Geographic location

West bounding longitude

East bounding longitude

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Temporal reference

Temporal extent

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End position

Dataset reference date

date type

publication

effective date

2011-07-01T00:00:00Z

Frequency of update

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Conformity

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version of format

Constraints related to access and use

Constraint set

Use constraints

Limitations on public access

None

Responsible organisations

Responsible party

contact position

OpenSky Support

organisation name

UCAR/NCAR - Library

full postal address

PO Box 3000

Boulder

80307-3000

email address

opensky@ucar.edu

web address

http://opensky.ucar.edu/

name: homepage

responsible party role

pointOfContact

Metadata on metadata

Metadata point of contact