Injection of iodine to the stratosphere
We report a new estimation of the injection of iodine into the stratosphere based on novel daytime (solar zenith angle < 45°) aircraft observations in the tropical tropopause layer and a global atmospheric model with the most recent knowledge about iodine photochemistry. The results indicate that significant levels of total reactive iodine (0.25-0.7 parts per trillion by volume), between 2 and 5 times larger than the accepted upper limits, can be injected into the stratosphere via tropical convective outflow. At these iodine levels, modeled iodine catalytic cycles account for up to 30% of the contemporary ozone loss in the tropical lower stratosphere and can exert a stratospheric ozone depletion potential equivalent to, or even larger than, that of very short-lived bromocarbons. Therefore, we suggest that iodine sources and chemistry need to be considered in assessments of the historical and future evolution of the stratospheric ozone layer.
document
http://n2t.net/ark:/85065/d7g73g2q
eng
geoscientificInformation
Text
publication
2016-01-01T00:00:00Z
publication
2015-08-01T00:00:00Z
Copyright 2015 American Geophysical Union.
None
OpenSky Support
UCAR/NCAR - Library
PO Box 3000
Boulder
80307-3000
name: homepage
pointOfContact
OpenSky Support
UCAR/NCAR - Library
PO Box 3000
Boulder
80307-3000
name: homepage
pointOfContact
2023-08-18T19:04:15.458215