Identification

Title

Assessment of source contributions to seasonal vegetative exposure to ozone in the U.S.

Abstract

W126 is a cumulative ozone exposure index based on sigmoidally weighted daytime ozone concentrations used to evaluate the impacts of ozone on vegetation. We quantify W126 in the U.S. in the absence of North American anthropogenic emissions (North American background or "NAB") using three regional or global chemical transport models for May-July 2010. All models overestimate W126 in the eastern U.S. due to a persistent bias in daytime ozone, while the models are relatively unbiased in California and the Intermountain West. Substantial difference in the magnitude and spatial and temporal variability of the estimates of W126 NAB between models supports the need for a multimodel approach. While the average NAB contribution to daytime ozone in the Intermountain West is 64-78%, the average W126 NAB is only 9-27% of current levels, owing to the weight given to high O₃ concentrations in W126. Based on a three-model mean, NAB explains ∼30% of the daily variability in the W126 daily index in the Intermountain West. Adjoint sensitivity analysis shows that nationwide W126 is influenced most by NOx emissions from anthropogenic (58% of the total sensitivity) and natural (25%) sources followed by nonmethane volatile organic compounds (10%) and CO (7%). Most of the influence of anthropogenic NOx comes from the U.S. (80%), followed by Canada (9%), Mexico (4%), and China (3%). Thus, long-range transport of pollution has a relatively small impact on W126 in the U.S., and domestic emissions control should be effective for reducing W126 levels.

Resource type

document

Resource locator

Unique resource identifier

code

http://n2t.net/ark:/85065/d7c24xbd

codeSpace

Dataset language

eng

Spatial reference system

code identifying the spatial reference system

Classification of spatial data and services

Topic category

geoscientificInformation

Keywords

Keyword set

keyword value

Text

originating controlled vocabulary

title

Resource Type

reference date

date type

publication

effective date

2016-01-01T00:00:00Z

Geographic location

West bounding longitude

East bounding longitude

North bounding latitude

South bounding latitude

Temporal reference

Temporal extent

Begin position

End position

Dataset reference date

date type

publication

effective date

2014-01-16T00:00:00Z

Frequency of update

Quality and validity

Lineage

Conformity

Data format

name of format

version of format

Constraints related to access and use

Constraint set

Use constraints

Limitations on public access

None

Responsible organisations

Responsible party

contact position

OpenSky Support

organisation name

UCAR/NCAR - Library

full postal address

PO Box 3000

Boulder

80307-3000

email address

opensky@ucar.edu

web address

http://opensky.ucar.edu/

name: homepage

responsible party role

pointOfContact

Metadata on metadata

Metadata point of contact