Multiple new-particle growth pathways observed at the US DOE Southern Great Plains field site

New-particle formation (NPF) is a significant source of aerosol particles into the atmosphere. However, these particles are initially too small to have climatic importance and must grow, primarily through net uptake of lowvolatility species, from diameters similar to 1 to 30-100 nm in order to potentially impact climate. There are currently uncertainties in the physical and chemical processes associated with the growth of these freshly formed particles that lead to uncertainties in aerosol-climate modeling. Four main pathways for new-particle growth have been identified: condensation of sulfuric-acid vapor (and associated bases when available), condensation of organic vapors, uptake of organic acids through acid-base chemistry in the particle phase, and accretion of organic molecules in the particle phase to create a lower-volatility compound that then contributes to the aerosol mass. The relative importance of each pathway is uncertain and is the focus of this work.

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Copyright Author(s) 2016. This work is distributed under the Creative Commons Attribution 3.0 License.


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Author Hodshire, Anna L.
Lawler, Michael J.
Zhao, Jun
Ortega, John
Jen, Coty
Yli-Juuti, Taina
Brewer, Jared F.
Kodros, Jack K.
Barsanti, Kelley C.
Hanson, Dave R.
McMurry, Peter H.
Smith, James N.
Pierce, Jeffery R.
Publisher UCAR/NCAR - Library
Publication Date 2016-07-28T00:00:00
Digital Object Identifier (DOI) Not Assigned
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Topic Category geoscientificInformation
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Metadata Date 2023-08-18T18:25:53.787055
Metadata Record Identifier edu.ucar.opensky::articles:18827
Metadata Language eng; USA
Suggested Citation Hodshire, Anna L., Lawler, Michael J., Zhao, Jun, Ortega, John, Jen, Coty, Yli-Juuti, Taina, Brewer, Jared F., Kodros, Jack K., Barsanti, Kelley C., Hanson, Dave R., McMurry, Peter H., Smith, James N., Pierce, Jeffery R.. (2016). Multiple new-particle growth pathways observed at the US DOE Southern Great Plains field site. UCAR/NCAR - Library. http://n2t.net/ark:/85065/d7sn0bng. Accessed 23 June 2025.

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