N2o temporal variability from the middle troposphere to the middle stratosphere based on airborne and balloon-borne observations during the period 1987-2018

Nitrous oxide (N2O) is the fourth most important greenhouse gas in the atmosphere and is considered the most important current source gas emission for global stratospheric ozone depletion (O-3). It has natural and anthropogenic sources, mainly as an unintended by-product of food production activities. This work examines the identification and quantification of trends in the N2O concentration from the middle troposphere to the middle stratosphere (MTMS) by in situ and remote sensing observations. The temporal variability of N2O is addressed using a comprehensive dataset of in situ and remote sensing N2O concentrations based on aircraft and balloon measurements in the MTMS from 1987 to 2018. We determine N2O trends in the MTMS, based on observations. This consistent dataset was also used to study the N2O seasonal cycle to investigate the relationship between abundances and its emission sources through zonal means. The results show a long-term increase in global N2O concentration in the MTMS with an average of 0.89 +/- 0.07 ppb/yr in the troposphere and 0.96 +/- 0.15 ppb/yr in the stratosphere, consistent with 0.80 ppb/yr derived from ground-based measurements and 0.799 +/- 0.024 ppb/yr ACE-FTS (Atmospheric Chemistry Experiment Fourier Transform Spectrometer) satellite measurements.

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Related Dataset #1 : N2O mixing ratio zonal mean and trend in the UTLS from aircraft and balloon measurements
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Author Krysztofiak, G.
Catoire, V.
Dudok de Wit, T.
Kinnison, Douglas E.
Ravishankara, A. R.
Brocchi, V.
Atlas, E.
Bozem, H.
Commane, R.
D'Amato, F.
Daube, B.
Diskin, G. S.
Engel, A.
Friedl-Vallon, F.
Hintsa, E.
Hurst, D. F.
Hoor, P.
Jegou, F.
Jucks, K. W.
Kleinböhl, A.
Küllmann, H.
Kort, E. A.
McKain, K.
Moore, F. L.
Obersteiner, F.
Ramos, Y. G.
Schuck, T.
Toon, G. C.
Viciani, S.
Wetzel, G.
Williams, J.
Wofsy, S. C.
Publisher UCAR/NCAR - Library
Publication Date 2023-03-18T00:00:00
Digital Object Identifier (DOI) Not Assigned
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Topic Category geoscientificInformation
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Metadata Date 2025-07-11T15:53:30.199906
Metadata Record Identifier edu.ucar.opensky::articles:26437
Metadata Language eng; USA
Suggested Citation Krysztofiak, G., Catoire, V., Dudok de Wit, T., Kinnison, Douglas E., Ravishankara, A. R., Brocchi, V., Atlas, E., Bozem, H., Commane, R., D'Amato, F., Daube, B., Diskin, G. S., Engel, A., Friedl-Vallon, F., Hintsa, E., Hurst, D. F., Hoor, P., Jegou, F., Jucks, K. W., Kleinböhl, A., Küllmann, H., Kort, E. A., McKain, K., Moore, F. L., Obersteiner, F., Ramos, Y. G., Schuck, T., Toon, G. C., Viciani, S., Wetzel, G., Williams, J., Wofsy, S. C.. (2023). N2o temporal variability from the middle troposphere to the middle stratosphere based on airborne and balloon-borne observations during the period 1987-2018. UCAR/NCAR - Library. https://n2t.org/ark:/85065/d7v4107s. Accessed 02 August 2025.

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